C G Deshpande
Articles written in Journal of Earth System Science
Volume 113 Issue 1 March 2004 pp 1-25
Measurements of the submicron aerosol size distribution made at the Indian Antarctic station, Maitri (70‡45′S, 11‡44′E) from January 10th to February 24th, 1997, are reported. Total aerosol concentrations normally range from 800 to 1200 particles cm−3 which are typical values for the coastal stations at Antarctica in summer. Aerosol size distributions are generally trimodal and open-ended with a peak between 75 and 133 nm and two minima at 42 and 420 nm. Size distributions remain almost similar for several hours or even days in absence of any meteorological disturbance. Total aerosol concentration increases by approximately an order of magnitude whenever a low pressure system passes over the station. Based on the evolution of aerosol size-distributions during such aerosol enhancement periods, three types of cases have been identified. The nucleation mode in all three cases has been suggested to result from the photochemical conversion of the DMS emissions transported either by the marine air or by the air from the ice-melt regions around Maitri. Subsidence of midtropospheric air during the weakening of radiative inversion is suggested as a possible source of the nucleation mode particles in the third case. Growth of the nucleation mode particles by condensation, coagulation and/or by cloud processes has been suggested to be responsible for other modes in size distributions.
Volume 119 Issue 4 August 2010 pp 479-487
Measurements of the concentration and size distribution of aerosol particles in the size-ranges of 0.5–20 𝜇 m and 16–700 nm diameters were made during six fog episodes over the south Indian Ocean. Observations show that concentrations of particles of all sizes start decreasing 1–2 hours before the occurrence of fog. This decrease is more prominent for coarse particles of < 1 𝜇 m diameter and continues until 10–20 minutes before the onset of fog when particle concentrations in all size ranges rapidly increase by one/two orders of magnitude in ∼20 minutes. Thereafter, concentrations of particles of all sizes gradually decrease until the dissipation of fog. After the fog dissipation, concentrations of coarse mode particles rapidly increase and restore to their pre-fog levels but concentrations of the Aitken mode particles decrease slowly and reach their pre-fog levels only after 1–2 hours. The net effect of fog is to change the bimodal size distributions of aerosols with a coarse mode at 1.0 𝜇 m and an accumulation mode at 40–60 nm to a power law size distribution. It is proposed that the preferential growth and sedimentation of the coarse mode hygroscopic particles in the initial phase cause a large decrease in the aerosol surface area. As a result, the low vapour pressure gases which were initially being used for the growth of coarse mode particles, now accelerate the growth rates of the accumulation and Aitken mode particles.
Volume 123 Issue 1 February 2014 pp 201-212
Measurements of the number concentration and size distribution of aerosol particles in the size range of 0.5–20 𝜇m diameter were made with an aerodynamic particle sizer at an Arctic site at Ny-Alesund, Svalbard in August–September 2007 during the International Polar Year 2007–2008. Data are analyzed to study the aerosol number concentration–wind speed relationships. The sea-salt particles of marine origin generated within the Arctic circle are identified as the main source of the Arctic summer aerosols. Total number concentration of aerosol particles increases with increase in wind speed, the increase being more when winds from open leads over the oceanic sector are reaching the station as compared to when winds from pack ice in other directions are reaching the station. The larger increase with winds from the oceanic sector is attributed to the enhanced bubble-breaking activity and increased entrainment of dimethyl sulphide particles at the sea surface. Although, the increase in total aerosol number concentration associated with the winds from the oceanic sector is spread over the whole range of particle sizes, the increase in coarse mode particles is more prominent than that in the accumulation mode particles. The age of airmass over pack ice is also an important factor to determine the aerosol concentration over the Arctic region. The process of rainout/washout of the aerosol particles due to drizzle/snowfall is an effective sink mechanism in the Arctic environment. The aerosol particle concentration starts decreasing within a few minutes from the start of these events but requires a few hours to restore to the normal background aerosol level after the end of event.